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Palladium(0)-Catalyzed Cope Rearrangement of Acyclic 1,5-Dienes. Bis(π-allyl)palladium(II) Intermediate

✍ Scribed by Nakamura, Hiroyuki; Iwama, Hideki; Ito, Masateru; Yamamoto, Yoshinori

Book ID
126942017
Publisher
American Chemical Society
Year
1999
Tongue
English
Weight
116 KB
Volume
121
Category
Article
ISSN
0002-7863

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ChemInform Abstract: Palladium(0)-Cataly
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Evidence for (π-allyl)palladium(II)(quin
Evidence for (π-allyl)palladium(II)(quinone) complexes in the palladium-catalyzed 1,4-diacetoxylation of conjugated dienes
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Evidence for a coordination of p-benxoquinone to palladium in [4-acetoxy-n3-(1,2,3)-cyclohexenyllpalladium(II) complexes was provided by changes of the 'H NMR chemical shift values of the r-ally1 protons and a decrease of the spin-lattice relaxation time constant for the p-benxoquinone protons. We h