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Mechanistic aspects of transition metal catalysed 1,6-diene and 1,6-enyne cycloisomerisation reactions

โœ Scribed by Lloyd-Jones, Guy C.

Book ID
118041010
Publisher
Royal Society of Chemistry
Year
2002
Tongue
English
Weight
699 KB
Volume
1
Category
Article
ISSN
1477-0520

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## Abstract The mechanism of the highly regioselective cycloisomerisation of dimethyl heptโ€1,6โ€dienylโ€4,4โ€dicarboxylate (1) by a neutral preโ€catalyst, [(__t__BuCN)~2~PdCl~2~] (8), to generate dimethyl 3,4โ€dimethylcyclopentโ€2โ€eneโ€1,1โ€dicarboxylate (3) has been investigated by isotopic labelling (rea