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Kinetics of the reactions of substituted benzoquinones with alkyl radicals

✍ Scribed by I. A. Shlyapnikova; V. A. Roginskii; V. B. Miller

Book ID
112441964
Publisher
Springer
Year
1978
Tongue
English
Weight
322 KB
Volume
27
Category
Article
ISSN
1573-9171

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Relative rate constants for the reactions of hydroxyl radicals with a series of alkyl substituted olefins were measured by competitive reactions between pairs of olefins a t 298 r 2 K and 1 atmospheric pressure. Hydroxyl radicals were produced by the photolysis of H,O, with 254-nm irradiation. The o

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It is demonstrated that photohalogenations of low reactivity substrates with BrCl occurs mainly with Cl' selectivity. With tertiary or benzylic hydrogens in the substrate, mainly Br' selectivity is observed. These observations are rationalized, taking into account the relative concentrations of ha