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In situ UV-Vis spectroelectrochemical evidence of an EC mechanism in the electrooxidation of N-Methylaniline

✍ Scribed by Albertas Malinauskas; Rudolf Holze

Book ID: 112008773
Publisher: Wiley (John Wiley & Sons)
Year: 1997
Tongue: English
Weight: 551 KB
Volume: 101
Category: Article
ISSN: 0372-8323
DOI: 10.1002/bbpc.19971011210

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We wish to report direct evidence for a homolytic scission-recombination mechanism in the thermal eMeisenheimer" rearrangement' of the title compound, I, to the hydroxylamine, II (equation I). This mechanism W&B apparently first proposed by Schgllkopf,3 who adduced threefold