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Impulsive excitation of pseudo-rotation for geometric phase detection

โœ Scribed by Jeffrey A. Cina

Publisher
John Wiley and Sons
Year
2000
Tongue
English
Weight
50 KB
Volume
31
Category
Article
ISSN
0377-0486

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โœฆ Synopsis

The prospects for using electronically resonant impulsive stimulated Raman scattering (ISRS) to prepare coherent molecular pseudo-rotation were investigated. Large-amplitude pseudo-rotation is a prerequisite for time-resolved optical measurement of electronic Berry-phase development according to a scheme proposed previously. It is shown that resonant ISRS should readily be able to generate the pseudo-rotating states needed for wave-packet interferometry experiments of that kind.

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