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Ground-state rotational constants of Ar+3 by rotational depletion coherence spectroscopy

✍ Scribed by Thomas F. Magnera; Douglas M. Sammond; Josef Michl

Book ID: 103033810
Publisher: Elsevier Science
Year: 1993
Tongue: English
Weight: 281 KB
Volume: 211
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(93)87076-f

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✦ Synopsis

Rotational depletion coherence spectroscopy permits the determination of ground-state rotational constants of photodissociable ions from orientation recurrences observed for the remaining ions after substantial depletion by a linearly polarized ps pulse of light at wavelengths absorbed by the ions. The method is complementary to ordinary rotational coherence spectroscopy. It has ken tested on the 4oArz and 36Ar$ ions, whose rotational constants are (9.0k0.2) x 10' s-' and (10.0k0.2) X 10' s-l, respectively.

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