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Golden rule calculation of product vibronic population inversions in photodissociation and related reactions

✍ Scribed by Michael J. Berry

Publisher: Elsevier Science
Year: 1974
Tongue: English
Weight: 817 KB
Volume: 29
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(74)85117-1

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✦ Synopsis

An ultrasimple reaction dyr?amics model successfully trcat~ product vibronic state distributions in photodissociation and predissociation reactions and in collision-induced electronic-to-kibrntiod energy transfer grocesses. product vibronic populgion inversions are determinen by intrairagment dynamics (i.e., changes in bond lengths m_~t strequtis) which occur ,during reaction product forma&n.

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Golden rule calculation of reaction prod

Golden rule calculation of reaction product vibronic state distributions

✍ Michael J. Berry 📂 Article 📅 1974 🏛 Elsevier Science 🌐 English ⚖ 454 KB

A resonrmce decay model of bimolecular exchange reactions successfully treats product vibronic stale distributions. Product vibronic population inversions are controlled by the extent of product structural change whichoccurs as reaction energy is released.