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From a Biogenetic Scenario to a Synthesis of the ABC Ring of Manzamine A

✍ Scribed by Herdemann, Matthias; Al-Mourabit, Ali; Martin, Marie-Thérèse; Marazano, Christian

Book ID
120165128
Publisher
American Chemical Society
Year
2002
Tongue
English
Weight
124 KB
Volume
67
Category
Article
ISSN
0022-3263

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The first total synthesis of haliclamine A (1), a macrocyclic marine alkaloid closely related to the key bisdihydropyridine intermediate 3 of the biogenetically unique manzamine family, has been efficiently achieved via stepwise inter-and intramolecular N-alkylations of 3-alkylpyridine derivatives 2