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Franck—Condon breakdown as a probe of continuum coupling in molecular photoionization

✍ Scribed by Sandeep Kakar; Heung Cheun Choi; E.D. Poliakoff

Book ID: 103035323
Publisher: Elsevier Science
Year: 1992
Tongue: English
Weight: 295 KB
Volume: 190
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(92)85178-d

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✦ Synopsis

We have measured vibrational branching ratios for 4t~-~ photoionization of CO in order to characterize continuum channel coupling. The results indicate that the shape resonance in the 5o--,~t~ channel influences vibrational branching ratios of the 4ochannel via continuum coupling, and the data illustrate how continuum channel coupling affects molecular photoionization dynamics.

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