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Extended Scope of Dirhodium(II)-Catalyzed Enantioselective Intramolecular 1,3-Dipolar Cycloadditions of Carbonyl Ylides with Alkene and Alkyne Dipolarophiles.

✍ Scribed by David M. Hodgson; Agnes H. Labande; Francoise Y. T. M. Pierard

Publisher: John Wiley and Sons
Year: 2003
Weight: 127 KB
Volume: 34
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.200315038

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## Abstract The first successful example of the enantioselective intermolecular 1,3‐dipolar cycloaddition of a chiral dirhodium(II) catalyst‐associated carbonyl ylide with an aromatic aldehyde dipolarophile is described. The tandem carbonyl ylide formation/cycloaddition reactions of 1‐diazo‐5‐aryl‐