✦ LIBER ✦

Energy deposition in SO2 via intense infrared laser multiphoton excitation

✍ Scribed by James V. Tietz; Shih-I Chu

Publisher: Elsevier Science
Year: 1983
Tongue: English
Weight: 519 KB
Volume: 101
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(83)87511-3

No coin nor oath required. For personal study only.

✦ Synopsis

The feasibility of multiphoton exitaton (MPE) and dissociation (hiPD) of trktomic molecules is the subject of current e~perimenral controversy_ The most probable path approximation (MPPA) makes use of artificial intelligence algorithms to select the most important excitation paths within the semiclassical Floquet matrix, allowing efticient and accurate cakulation of non-linear SIPE quantum dynamics to very high order. An zb initio study of SOa using the MPPA indicates thnt collisionless MPD xxill not be achieved at laser field strengths under 20 GW/cm'. The possibility of hlPD at higher laser intensities is currently under imestigation.

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