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Effects of Solvent and Solute Polarizability on the Reorganization Energy of Electron Transfer

✍ Scribed by Gupta, Shikha; Matyushov, Dmitry V.

Book ID
126869053
Publisher
American Chemical Society
Year
2004
Tongue
English
Weight
116 KB
Volume
108
Category
Article
ISSN
1089-5639

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✍ Yoshitaka Enomoto; Toshiaki Kakitani; Akira Yoshimori; Yasuyo Hatano πŸ“‚ Article πŸ“… 1991 πŸ› Elsevier Science 🌐 English βš– 444 KB

We conducted Monte Carlo simulations of polar solutions by explicitly treating the effect of electronic polarizability of solvent molecules. Based on these data, we calculated the energy-gap dependence of electron-transfer rates. It was found that a considerable asymmetry of the energy-gap dependenc