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Effect of three-body interactions on the early stages of atomic cluster growth

✍ Scribed by I.L. Garzón; Estela Blaisten-Barojas

Publisher
Elsevier Science
Year
1986
Tongue
English
Weight
460 KB
Volume
124
Category
Article
ISSN
0009-2614

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✦ Synopsis

The sequence of conformatlons a cluster assumes as it grows from a trimer into a thirteen-atom aggregrate under a given model potential has been studied. The model potential proposed is a construction composed of a van der Waals pairwise term and a three-body term composed of the triple dipole contribution and the exchange overlap contribution.

A parametric study of the thermodynamically preferred structures is given. After reaching a boundary between regions in the parameter space, equilibrium mixtures of isomers with different packings are obtained. The normal frequency spectrum is given for clusters up to thirteen atoms.

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