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Divergent Construction of Nitrogen-Containing Polycyclic Compounds with a Dearomatization Strategy

✍ Scribed by Wang, Linfei; Fan, Renhua

Book ID
127303325
Publisher
American Chemical Society
Year
2012
Tongue
English
Weight
267 KB
Volume
14
Category
Article
ISSN
1523-7060

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Nitroethylenes bearing either a phenylthio or a phenylselenoether group in b-position are efficient synthetic equivalents of nitroacetylene. A [4+2] cycloaddition/carbenoid-mediated elimination of PhS(e)CH 3 /[4+2] cycloaddition sequence of reactions is shown to produce formal biscycloadducts of nit