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Diels−Alder Reactions and the Structure of Transition States

✍ Scribed by Coleman, William F.

Book ID: 119997928
Publisher: American Chemical Society
Year: 2010
Tongue: English
Weight: 904 KB
Volume: 87
Category: Article
ISSN: 0021-9584
DOI: 10.1021/ed1009078

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We have recently determined kinetic parameters for the unimolecular Diels-Alder retrogressions of exe and w-dicyclopentadiene to monomer (1). The activation enthalpies and entropies are aH f (E) 37.4 2 0.3 kcal/mole, hSS (E) + 1.1 2 0.6 e.u., hH + (&) 33.0 2 0.5 kcal/mole, and hSS (endo) \_ -1.9 +