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Diastereoselective Multicomponent Cyclizations of Fischer Carbene Complexes, Lithium Enolates, and Allylmagnesium Bromide Leading to Highly Substituted Five- and Six-Membered Carbocycles.

✍ Scribed by Jose Barluenga; Ivan Perez-Sanchez; Marcos G. Suero; Eduardo Rubio; Josefa Florez

Publisher: John Wiley and Sons
Year: 2007
Weight: 47 KB
Volume: 38
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.200703066

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## Abstract β‐Substituted alkenylcarbene complexes react with methyl ketone lithium enolates to give different carbocyclization products depending on the structure of the lithium enolate, on the metal of the carbene complex, and on the reaction media. Thus, the reactions of aryl and alkyl methyl ke