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Comparison of quantum mechanical and semiclassical cross sections and rate constants for vibrational relaxation of N2 and CO colliding with 4He

✍ Scribed by Gert Due Billing

Publisher: Elsevier Science
Year: 1986
Tongue: English
Weight: 632 KB
Volume: 107
Category: Article
ISSN: 0301-0104
DOI: 10.1016/0301-0104(86)85057-1

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A semiclassical collision modei has been irscd to cafcuhite the rate constant for vibrational reltxrtion in HD fu = 1, j = 0) colIid~ag with 4tie. The He + HD potential surface was obtained from an analyticat He + Hz surface previousfy used for similar c~caIatjons on NC f Hz and He + Dz\_ The fheorc

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✍ A. Plain; J. Jolly 📂 Article 📅 1987 🏛 Elsevier Science 🌐 English ⚖ 363 KB

A tunable dye laser was used to populate selectively a single rotational-vibrational state of N 2 ( B 'E , u' = 0, N' = O-l 5 ) . The population changes induced by collisions with He were determined using time-resolved spectroscopy in a flowing afterglow experiment. Total rotational transfer rates f

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Fully converged quantum cross sections for 4He-D2 (u= l,i=O) vibrational reliaxation were determined using the coupled-states method and a modikied version of the Gordon-Secrcst surface. First-order forbidden rotational transitions play a si@fkant role, comparable to that observed previously for the