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ChemInform Abstract: Enantiospecific Total Synthesis of (+)-2-Pupukeanone.

✍ Scribed by A. SRIKRISHNA; T. J. REDDY

Publisher: John Wiley and Sons
Year: 2010
Weight: 37 KB
Volume: 29
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.199813155

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✦ Synopsis

Enantiospecific Total Synthesis of (+)-2-Pupukeanone.

-The first enantiospecific total synthesis of 2-pupukeanone (X) starting from readily available (R)-carvone (I) is described. Key step in the synthetic sequence is the construction of the tricyclic isotwistane carbon framework via 5-exo-trig radical cyclization of the bicyclic compound (V). -(SRIKRISHNA, A.; REDDY,

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