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Atom-diatom scattering in the presence of reactive channels

✍ Scribed by E. Ficocelli Varracchio

Book ID
112832591
Publisher
Springer-Verlag,Italian Physical Society
Year
1981
Weight
285 KB
Volume
63
Category
Article
ISSN
0369-3554

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📜 SIMILAR VOLUMES

Effective potential theory of atom–diato
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✍ E. Ficocelli Varracchio 📂 Article 📅 1981 🏛 John Wiley and Sons 🌐 English ⚖ 710 KB

## Abstract A field‐theoretical formalism is applied to the problem of atom–diatom scattering, in the presence of “intermediate” reactive channels. This leads to an integral equation formulation for elastic processes and to a numerical quadrature problem for inelastic vibro–rotational transitions.

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An approximate method of Sakimoto and Onda for deriving the Smatrix elements for dissociative collisions in collinear atom-diatom reactive systems, which provided accurate total dissociation probabilities, has been tested further. To do this, kinetic energy distributions of atomic products have been

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Resonances in slow molecular collisions are demonstrated by exact numerical solution of the closecoupled'equations for r&&ion4 excitation. including closed channels. The breakdown of the adiabatic approximation is exhibited. Resonance energies can be essentially predicte-a by a "best local" approxim