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σ-Bond Metathesis of Alkanes on a Silica-Supported Tantalum(V) Alkyl Alkylidene Complex: First Evidence for Alkane Cross-Metathesis

✍ Scribed by Christophe Copéret; Olivier Maury; Jean Thivolle-Cazat; Jean-Marie Basset


Book ID
101368050
Publisher
John Wiley and Sons
Year
2001
Tongue
English
Weight
120 KB
Volume
113
Category
Article
ISSN
0044-8249

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σ-Bond Metathesis of Alkanes on a Silica
✍ Christophe Copéret; Olivier Maury; Jean Thivolle-Cazat; Jean-Marie Basset 📂 Article 📅 2001 🏛 John Wiley and Sons 🌐 English ⚖ 119 KB

C-C activation of unactivated alkanes on a silica-supported neopentyl neopentylidene Ta complex [Eq. (1)] affords the alkane cross-metathesis products tBuCH R and an alkane-metathesis catalyst. Since the activity and product distributions are similar to those obtained with a silica-supported Ta hydr