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α– Alums: K,Rb,Tl and NH4Al(SO4)2·12H2O – a new family of χ(3)-active crystalline materials for Raman laser converters with large frequency shifts

✍ Scribed by A. A. Kaminskii; E. Haussühl; S. Haussühl; H. J. Eichler; K. Ueda; J. Hanuza; K. Takaichi; H. Rhee; G. M. A. Gad


Publisher
John Wiley and Sons
Year
2004
Tongue
English
Weight
303 KB
Volume
1
Category
Article
ISSN
1612-2011

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✦ Synopsis


Efficient high-order stimulated Raman scattering was excited under picosecond pumping in the visible and near-IR in four crystals of the α-alum family - novel isotropic χ^(3)^-active crystalline materials. All observed Stokes and anti-Stokes lasing components were identified and attributed to the promoting ≈1000 cm^-1^vibration modes of these crystals. Their one-micron steady-state first Stokes Raman gain coefficients were estimated as well.