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Zur elektronenstruktur metallorganischer komplexe der ƒ-elemente—XXIV. Interpretation der optischen und magnetochemischen Eigenschaften von Cp3CeIII THF auf der Grundlage der kristallfeldtheorie

✍ Scribed by H. Reddmann; H. Schultze; H.-D. Amberger; C. Apostolidis; B. Kanellakopulos


Publisher
Elsevier Science
Year
1990
Tongue
English
Weight
594 KB
Volume
46
Category
Article
ISSN
1386-1425

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✦ Synopsis


On

the basis of magnetic susceptibility, NMR spectroscopic and optical measurements the crystal field splitting pattern of ($-C,H&Ce 'n*THF could be derived. The free parameters of an empirical Hamiltonian were fitted to the experimentally derived crystal field splitting pattern. Making use of the calculated crystal field eigenvalues, the magnetochemical data could be reproduced in a satisfactory manner.