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Yttrium Complexes as Catalysts for Living and Immortal Polymerization of Lactide to Highly Heterotactic PLA

✍ Scribed by Abderramane Amgoune; Christophe M. Thomas; Jean-François Carpentier


Publisher
John Wiley and Sons
Year
2007
Tongue
English
Weight
157 KB
Volume
28
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

Amino‐alkoxy‐bis(phenolate) yttrium complexes act in the presence of an excess of alcohol (up to 50 equiv. vs. Y) as highly active and stereoselective catalysts for rac‐lactide and racβ‐butyrolactone polymerizations. These versatile systems enable the production of large quantities of polymer with small amounts of catalyst, optimizing productivity, and also allow the preparation of polymers with functional end groups, which may be employed as intermediates for macromolecular engineering applications.

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