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Y-doped BaCeO3−δ nanopowders as proton-conducting electrolyte materials for ethane fuel cells to co-generate ethylene and electricity

✍ Scribed by Xian-Zhu Fu; Jing-Li Luo; Alan R. Sanger; Nancy Luo; Karl T. Chuang


Publisher
Elsevier Science
Year
2010
Tongue
English
Weight
967 KB
Volume
195
Category
Article
ISSN
0378-7753

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✦ Synopsis


Y-doped BaCeO 3-ı (BCY) powders synthesized using a combustion method are pure perovskite phases. The particles are uniform spherical particles about 50 nm. The properties of BCY proton-conducting electrolyte sintered at different temperatures from pressed nanopowders were systematically investigated. Dense BCY pellets are obtained at temperatures higher than 1400 • C for 10 h. Electrical conductivity and resistance to CO 2 atmosphere each increase with sintering temperature. Fuel cells having about 0.8 mm thick BCY electrolyte and Pt electrodes co-produce 151 mW cm -2 electrical power and value-added ethylene with selectivity over 90% at ethane conversion about 35% at 700 • C.