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Water-Soluble Triphenylphosphane-3,3′,3′′-tricarboxylate (m-TPPTC) Ligand and Methylated Cyclodextrins: A New Combination for Biphasic Rhodium-Catalyzed Hydroformylation of Higher Olefins

✍ Scribed by Sébastien Tilloy; Emilie Genin; Frédéric Hapiot; David Landy; Sophie Fourmentin; Jean-Pierre Genêt; Véronique Michelet; Eric Monflier


Publisher
John Wiley and Sons
Year
2006
Tongue
English
Weight
123 KB
Volume
348
Category
Article
ISSN
1615-4150

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✦ Synopsis


Abstract

The methylated cyclodextrins/m‐TPPTC [tris(m‐carboxyphenyl)phosphane trilithium salt] couples proved to be more efficient than the well‐known methylated cyclodextrins/TPPTS [tris(m‐sulfonatophenyl)phosphane trisodium salt] systems in terms of activities and selectivities to perform the Rh‐catalyzed hydroformylation of higher olefins in an aqueous‐organic system. The interactions cyclodextrins/m‐TPPTC have been fully studied by NMR spectroscopy.