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Visible-Light Excitation of Infrared Lanthanide Luminescence via Intra-Ligand Charge-Transfer State in 1,3-Diketonates Containing Push-Pull Chromophores

✍ Scribed by Nail M. Shavaleev; Rosario Scopelliti; Frédéric Gumy; Jean-Claude G. Bünzli


Book ID
102164810
Publisher
John Wiley and Sons
Year
2008
Tongue
English
Weight
208 KB
Volume
2008
Category
Article
ISSN
1434-1948

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✦ Synopsis


Abstract

A new 1,3‐diketonato ligand containing both an electron‐donor [4‐(dimethylamino)benzene] and an electron‐acceptor (4‐nitrobenzene) group and its lanthanide complexes have been prepared. They display an intense intra‐ligand charge‐transfer absorption transition in the visible region of the spectrum at 400–550 nm which was utilized to achieve visible‐light excitation of metal‐centred infrared luminescence of Nd^III^, Er^III^ and Yb^III^ ions. (© Wiley‐VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2008)