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Violet light second harmonic generation and optical properties of the nonlinear optical organometallic ZnCd(SCN)4 crystal

✍ Scribed by G.H Zhang; D Xu; Y.T Chow; M.K Lü; X.Q Wang; D.R Yuan; P.L Chu; Q Ren; X.G Xu

Publisher
Elsevier Science
Year
2004
Tongue
English
Weight
300 KB
Volume
233
Category
Article
ISSN
0030-4018

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✦ Synopsis

We report on continuous-wave violet-blue light generation by direct frequency doubling a laser diode in a ZnCd(SCN) 4 crystal. 10.3 mW second harmonic generation light at 404 nm is generated with a fundamental power of 1.46 W incident on 3-mm-long crystal. The d 14 , d 15 nonlinear optical coefficients of the crystal were also determined by the Maker fringes method at 1064 nm.

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## Abstract Bis(isothiocyanato)‐bis(4‐methylpyridine)zinc(II)(Zn(SCN)~2~(C~6~H~7~N)~2~), (abbreviated as ZBNC) single crystals of optical quality have been grown from acetone solution by the slow temperature‐lowering method. Its solubilities at different temperatures in acetone were measured. The X