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Vibrational energy redistribution of polyatomic molecules in liquids after ultrashort infrared excitation

✍ Scribed by K. Spanner; A. Laubereau; W. Kaiser

Publisher: Elsevier Science
Year: 1976
Tongue: English
Weight: 538 KB
Volume: 44
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(76)80415-0

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✦ Synopsis

Individual Ctf-~-strctchmg modes wcrc. cxcltcd by single tunable infrared pu!scs. l'hc gcncratcd cxccs population of the rnolcculcb was monitored by subscqucnt probe pulccs usmg spontaneous anti-Stokes R~mm scat Wing. ~xpcrirnental ddta JTL' xcported on ethanol &and CHsI iu solutions of CC1 4, Very rapid cncrgy transfer bctwccn neighboring v~bmtmn.d states is Jircctiy obbcrvcd.

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