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Vergleichende Untersuchung zur Diastereoselektivität derO-Methylierung von sterisch behinderten β-Ketocarbonsäureestern und ihren Enolen

✍ Scribed by Buß, Monika ;Meier, Herbert


Publisher
John Wiley and Sons
Year
1990
Tongue
English
Weight
216 KB
Volume
1990
Category
Article
ISSN
0947-3440

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✦ Synopsis


Diastereoselectivity of the O‐Methylation of Sterically Hindered β‐Ketocarboxylates and Their Enols

The enols 1a, b, and 1c, which exists almost completely in the keto form, have been methylated at the oxygen atom with diazomethane. The regioselective reaction can be catalyzed by methanol, but may loose in that case the diastereoselectivity. A comparison with the methylation of the enolates by iodomethane is discussed.