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Valence band formation in small silver clusters

โœ Scribed by G. Apai; S.-T. Lee; M.G. Mason

Publisher
Elsevier Science
Year
1981
Tongue
English
Weight
412 KB
Volume
37
Category
Article
ISSN
0038-1098

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๐Ÿ“œ SIMILAR VOLUMES

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The 4s and 3d ionization manifolds for Ni2 and Nia @ah) clusters are compared, usmg symmetry-broken SCF wavefunctions. The 4s ion states reman delo&tzed whereas each 3d eon hole is esscnt~ally loulued on a stnglc atom, thus causmg appreciable 4s polarization Slgticant overhp of 4s and 4d levels IS p

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The mean resonance energy (do> =R.fwwa(o) do/\_fu(o) dw calculated from the optical absorption spectra ofAg, in solid Ar shows strong variations as a function of cluster size, giving maxima at n =8,18 and 34. This behavior is discussed in terms of the electronic shell model. Static dipole polarizabi