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UV Laser Deposition of SiS/Poly(thiacarbosilane) Composites and their Conversion to SiO/Poly(thiacarbosiloxane) Composites

✍ Scribed by Radmila Tomovska; Markéta Urbanová; Jan Šubrt; Jaroslav Boháček; Josef Pola


Publisher
John Wiley and Sons
Year
2007
Tongue
English
Weight
328 KB
Volume
208
Category
Article
ISSN
1022-1352

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✦ Synopsis


Abstract

ArF laser irradiation of gaseous mixtures of carbon disulfide and silane allows efficient deposition of SiS bond‐containing poly(thiacarbosilanes) incorporating SiS bodies. These SiS/poly(thiacarbosilane) composites are the first example of silicon sulfide/polymer composites. Composite formation is analyzed by GC/MS analysis of volatile products and the structure of the composite as determined by electron microscopy and FT‐IR spectra. The composites undergo reaction with air moisture and methanol vapor, evolve H~2~S and evolve to nano‐sized poly(thiacarbosiloxane)s and poly(methoxythiacarbosiloxane)s.

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