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Using the comparison of steric versus electronic effects to infer mechanistic information in stepwise electrophilic addition reactions involving three-membered cyclic intermediates

✍ Scribed by Donna J. Nelson; Raman Soundararajan


Book ID
104217748
Publisher
Elsevier Science
Year
1988
Tongue
French
Weight
243 KB
Volume
29
Category
Article
ISSN
0040-4039

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✦ Synopsis


Correlations of 1% versus relative reactivities or formation constants of reactions of alkenes with ArSCl, MeCOSH. Ag+, or HgC12 reveal that complexation reactions show steric dependence, that additions with the first step rate-determining are sterically independent, and that those with the second step rate-determining are sterically dependent.

We recently reported a method of ascertaining the relative importance of steric and