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Uptake of copper ions by carbon fiber/polymer hybrids prepared by tandem diazonium salt chemistry and in situ atom transfer radical polymerization

✍ Scribed by Samia Mahouche Chergui; Nourredine Abbas; Tarik Matrab; Mireille Turmine; Elisabeth Bon Nguyen; Rémi Losno; Jean Pinson; Mohamed M. Chehimi


Publisher
Elsevier Science
Year
2010
Tongue
English
Weight
321 KB
Volume
48
Category
Article
ISSN
0008-6223

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✦ Synopsis


Cyclam-functionalized polyglycidyl methacrylate, grafted on carbon fibres (CF-PGMA-Cy) was prepared by atom transfer radical polymerization using aryl diazonium salt initiators.

These adsorption maximum capacity of CF-PGMA-Cy fibres for Cu(II) was found to be 28.6 mg/g at pH 5.2 and the adsorption kinetics fitted to the pseudo-second order model.

Cyclic voltammetry of the (CF-PGMA-Cy)-supported copper ions indicated true electrochemical stripping of Cu(II) with detection of as low as 2 pmol of adsorbed Cu 0 . CF-PGMA-Cy fibres are thus efficient and reusable adsorbents that hold promises for the design of electrochemical sensors of metal ions.