The homogeneous optical dephasing times (T,) and the non-photochemical hole burning (NPHB) linewidths of resorutin in glycerol glass are reported from 1.1 to 25.5 K. At low temperature, the linewidths obtained from NPHB are substantially wider than the linewidths (l/x T2) obtained from photon echo m
Unified theory of photon echoes: The passage from inhomogeneous to homogeneous line broadening
โ Scribed by Roger F. Loring; Shaul Mukamel
- Publisher
- Elsevier Science
- Year
- 1985
- Tongue
- English
- Weight
- 359 KB
- Volume
- 114
- Category
- Article
- ISSN
- 0009-2614
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โฆ Synopsis
WC cJlculate the temporal profllc of the photon echo signal from D collectIon of non-mtcractmg two-lcvcl s)'stems. whose frequcnclcs undergo Gauss~n random modulntlons The model IS cvvxiy solvable and mtcrpolatcs contmuously bct\wcn the mhomogeneous broadenrng hrnd tn which a wcll-dcfincd echo s&ma1 e\rsts and the homogeneous brondcnlng IunIt tn r\*htch It 1s no longer present The impbwtrons for the problem of conccntrat^londcpendent dephasmg m mixed molecular crystals arc dtscussed.
๐ SIMILAR VOLUMES
Experimental widths of high-n hydrogen Balmer lines H n (n = 6-12), emitted from a radiofrequency discharge (T = 1850 K and N e = 1.2 ร 10 13 cm -3 ), are systematically lower (up to 20%) than predicted by the Kepple-Griem (KG) line broadening theory [1]. This motivated a new theoretical analysis fo