We have made ultrasonic measurements on a filled skutterudite PrOs 4 Sb 12 showing a heavy Fermion superconductivity at T C ΒΌ 1:85 K: The elastic constants Γ°C 11 Γ C 12 Γ=2 and C 44 of PrOs 4 Sb 12 exhibit low-temperature softenings below 20 K down to T C ; indicating a quadrupole fluctuation of Pr
Ultrasonic dispersion and off-center rattling in heavy fermion superconductor
β Scribed by Yuichi Nemoto; Takafumi Ueno; Naoya Takeda; Takashi Yamaguchi; Tatsuya Yanagisawa; Terutaka Goto; Hitoshi Sugawara; Hideyuki Sato
- Publisher
- Elsevier Science
- Year
- 2006
- Tongue
- English
- Weight
- 168 KB
- Volume
- 378-380
- Category
- Article
- ISSN
- 0921-4526
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β¦ Synopsis
Ultrasonic attenuation measurements have been firstly performed for a large single crystal of PrOs 4 Sb 12 with the dimensions of 5:97 Γ 0:6 Γ 0:6 mm 3 . Remarkable frequency dependence around 20-40 K has been observed in the elastic constant and attenuation coefficient of the longitudinal C 11 mode associated with E g symmetry strain in part, which results from a thermally activated off-center rattling with E g symmetry of a Pr ion inside a Sb icosahedron cage. Parameters of a characteristic time t 0 ΒΌ 3:1 Γ 10 Γ11 s and an activation energy E ΒΌ 225 K were obtained. This E g rattling involving a local charge fluctuation inside a Sb cage periodically arranged may couple to the conduction electrons. As a result, the electron-phonon coupling would lead to heavy fermion and its superconductivity in PrOs 4 Sb 12 .
π SIMILAR VOLUMES
Ultrasonic investigation for the single crystals of ferromagnetic filled skutterudite compound NdOs 4 Sb 12 was performed. A marked frequency dependence of the ultrasonic dispersion has been observed in a longitudinal elastic constant C 11 at temperature centered around 45 K; however, no dispersion