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Ultrafast Laser Pulse Control of Exciton Dynamics: A Computational Study on the FMO Complex †

✍ Scribed by Brüggemann, Ben; May, Volkhard

Book ID
127010287
Publisher
American Chemical Society
Year
2004
Tongue
English
Weight
185 KB
Volume
108
Category
Article
ISSN
0022-3654

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By a wavepacket propagation, we demonstrate the possibility of controlling the photodissociation branching ratio between two fragment channels by a single ultrashort linearly chirped laser pulse. It is found that a negatively chirped pulse of a moderate chirp rate completely prohibits the production