Nitrogen atoms, as highly charged as N 5+, are found to be formed upon the irradiation of (NH3) . clusters with an intense femtosecond laser beam. Kinetic energy release values of the nitrogen atoms, from the Coulomb explosion of ammonia clusters, are found to be on the order of several hundred elec
Ultrafast laser-induced Coulomb explosion of clusters with high charge states
โ Scribed by J. Purnell; E.M. Snyder; S. Wei; A.W. Castleman Jr.
- Publisher
- Elsevier Science
- Year
- 1994
- Tongue
- English
- Weight
- 713 KB
- Volume
- 229
- Category
- Article
- ISSN
- 0009-2614
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โฆ Synopsis
Iodine and argon ions, as highly charged as I"+ and A?+, are found to be formed upon the irradiation of HI clusters and HIAr, clusters with an intense femtosecond laser beam. Double peaks are observed for each multicharged species, and identified to result from Coulomb explosion of clusters. Kinetic energy release values are calculated from the peak splittings, and also directly measured from cutoff potentials using a reflectron as an energy analyzer. The determined values are surprisingly large, on the order of several hundred electron volts.
๐ SIMILAR VOLUMES
Ablation of carbon clusters from a graphite surface exposed to 35 ps wide 1064 nm wavelength, laser pulses of intensities of the order of 1014 W cm 2 yields cluster ions in high charge states. Double and triple coincidence spectra of singly-charged atomic fragments resulting from spontaneous dissoci