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Two-Dimensional Marangoni-Instability-Induced Periodic Patterns of Polymer Blend Films Cast on Tilted Substrates

✍ Scribed by Kuen-Hua Wu; Shih-Yuan Lu; Hsin-Lung Chen; Yen-Yi Chen


Publisher
John Wiley and Sons
Year
2008
Tongue
English
Weight
438 KB
Volume
209
Category
Article
ISSN
1022-1352

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✦ Synopsis


Abstract

Two‐dimensional periodic patterns were observed for PS/PVP blend films and the corresponding homopolymer films on tilted glass substrates. They were attributed to the Marangoni instability resulting from surface tension non‐uniformity. For the 1:1 PS‐1/PVP‐1 blend films, two‐dimensional regular arrays of the separated phases were observed, similar to those observed on homopolymer films from thickness variations. In addition, for the PS‐2/PVP‐2 blend films of 30/70 composition, one‐dimensional strip patterns of separated phases were observed. The pattern formation mechanism is discussed and a characteristic parameter, defined as the ratio of the final film thickness to initial solution viscosity, is found to correlate well with the pattern regularity through variation in polymer concentration.

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