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Tris(trimethylsilyl)methane as an internal 13C NMR chemical shift thermometer

✍ Scribed by William H. Sikorski; Aaron W. Sanders; Hans J. Reich


Publisher
John Wiley and Sons
Year
1998
Tongue
English
Weight
228 KB
Volume
36
Category
Article
ISSN
0749-1581

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✦ Synopsis


Tris(trimethylsilyl)methane has excellent properties for an internal chemical shift thermometer to measure temperatures in 13C DNMR spectroscopy [*d between the 13C signals of and CH carbons]. It is Si(CH 3

) 3 chemically inert, soluble in most organic solvents and has an almost linear dependence of *d on temperature. The sensitivity (approximately 1 ¡C Hz~1 at 90 MHz) allows the measurement of temperature to within 1 ¡C. The chemical shift is solvent dependent, so each solvent mixture must be calibrated. Calibrations are presented for seven solvents.