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Triplet Excitation Transfer through the Walls of Hemicarcerands: Dependence of the Electronic Coupling on the Size of the Molecular Cage

โœ Scribed by Romanova, Zinaida S.; Deshayes, Kurt; Piotrowiak, Piotr

Book ID
127203337
Publisher
American Chemical Society
Year
2001
Tongue
English
Weight
212 KB
Volume
123
Category
Article
ISSN
0002-7863

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We analyze electronic radialionless transitions in molecular aggregates in the limit where the coupling between the monomeric units is strong. We show that in this limit the rate at a given electronic energy gap decreases drastically with the increase in zhe size of the system. The dccrcase becomes