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Transport and magnetotransport properties of cold-pressed CrO2 powder

โœ Scribed by Liu, H. ;Zheng, R. K. ;Wang, Y. ;Bai, H. L. ;Zhang, X. X.


Publisher
John Wiley and Sons
Year
2005
Tongue
English
Weight
230 KB
Volume
202
Category
Article
ISSN
0031-8965

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โœฆ Synopsis


Abstract

Resistivity of coldโ€pressed CrO~2~ powder has been measured over the temperature range of 2 to 350 K with a magnetic field up of to 50 kOe. High resolution transmission electron microscopy (HRTEM) images show that the CrO~2~ particles are needleโ€shaped with an aspect ratio of 7:1 and have an average length of 200 nm, and are covered with an ultraโ€thin (โˆผ2.5 nm) native Cr~2~O~3~ layer. Temperature dependent conductivity can be well described by the expression below 55 K, a feature of electron tunneling, and by the higherโ€order hopping for temperature above 55 K. The magnetoresistance, , reaches โˆผ33.5% at 2 K and decreases to nearly zero at room temperature. Temperature dependent saturation magnetization follows well the relation below 240 K. The spinโ€wave stiffness constant, D, is estimated to be โˆผ91 meV ร…^2^. By fitting the specific heat measured in the temperature range of 1.8โ€“34 K by the relation , we obtained the electronic specific heat coefficient ฮณ = 1.7 mJ/mol K^2^, this corresponds to a density of states at the Fermi level of 0.73 states/eV, which is in good accordance with the theoretical value of 0.69 states/eV.


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