Transient stimulated vibrational Raman scattering in liquid HCl, HBr, Cl2, CR, $0, CHsF, CH3Q and SF6 has been observed Using a mode-locked ruby laser. Efficient conversions to Stokes wavelengths (up to 10%) are observed resulting in large excitation of the vibrational population. Recent laser measu
Transient vibrational grating scattering
โ Scribed by D.P. Weitekamp; Koos Duppen; Douwe A. Wiersma
- Publisher
- Elsevier Science
- Year
- 1983
- Tongue
- English
- Weight
- 570 KB
- Volume
- 102
- Category
- Article
- ISSN
- 0009-2614
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โฆ Synopsis
A new method for measuring vibrational lifetimes in the solid state is demonstrated in a dilute mixed molecular crystal Using a picosecond light pulse at wr and simuJtaneous crossed pukes at r,+, a viirational population grating at wr -wa is prepared. The decay of this grating is followed by measuring at variable delay the Bragg-a@e diffraction of a probe pulse, resonant with an optical transition.
๐ SIMILAR VOLUMES
A novel modification of the forced Rayleigh scattering method for determining the translational diffusion coefficient and lifetime of photochromic moieties is effected through imposition of a nonsinusoidal transient optical sating flOt.2) to a condensed medium sample. A multiple~rder diffraction pat