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Toward the description of van der Waals interactions within density functional theory

✍ Scribed by Lein, M.; Dobson, J. F.; Gross, E. K. U.


Publisher
John Wiley and Sons
Year
1999
Tongue
English
Weight
201 KB
Volume
20
Category
Article
ISSN
0192-8651

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✦ Synopsis


On the basis of the adiabatic connection formula we propose several approximations for the total correlation energy functional, which, in the limit of two separated neutral subsystems, correctly reproduce the van der Waals R y6 behavior. We have calculated the corresponding van der Waals coefficients as well as total correlation energies, thus demonstrating the feasibility of a ''seamless'' functional.