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Time resolved study of vibrational relaxation in solid CO2 at high pressures

โœ Scribed by Michael Baggen; Ad Lagendijk

Publisher
Elsevier Science
Year
1991
Tongue
English
Weight
424 KB
Volume
177
Category
Article
ISSN
0009-2614

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โœฆ Synopsis

The vibrational coherence relaxation of the S2, bound state of the Fermi dyad vI:2v2 in solid CO2 is studied with the timeresolved stimulated Raman technique as a function of temperature for pressures up to 4.4 GPa. The relaxation is determined by a competition between two contributions: a down-conversion process with a weak pressure dependence, and a pure dephasing process, the latter becoming dominant at higher pressures.

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