A comparison of first hyperpolarizabilities /3 determined by hyper-Rayleigh scattering (HRS; /3HRS) and electric field-induced second-harmonic generation (EFISH; /3E~aSn) for a series of donor-acceptor substituted ~r-conjugated organic compounds shows a marked discrepancy between /3H~ and /3E~aSH va
✦ LIBER ✦
Time-resolved hyper-Rayleigh scattering: measuring first hyperpolarizabilities β of fluorescent molecules
✍ Scribed by O.F.J. Noordman; N.F. van Hulst
- Publisher
- Elsevier Science
- Year
- 1996
- Tongue
- English
- Weight
- 401 KB
- Volume
- 253
- Category
- Article
- ISSN
- 0009-2614
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We provide an improved method for measuring the first order hyperpolarizability of organic nonlinear optical materials in solution by the hyper-Rayleigh scattering technique. The method is free from the overestimation which is encountered in the conventional method due to the fluorescence induced by