We describe the results of a number of experiments which demonstrate competition between three-photon resonance-enhanced multiphoton ionisation and third-harmonic generation (THG) at wavelengths near the (= 'IT.-% 'Z.$ (rc: 4so,+x:) Rydberg transition of acetylene. The results serve to strengthen a
β¦ LIBER β¦
Third-harmonic generation and ionisation processes in Kr
β Scribed by M.J. Proctor; J.A.D. Stockdale; T. Efthimiopoulos; C. Fotakis
- Publisher
- Elsevier Science
- Year
- 1987
- Tongue
- English
- Weight
- 306 KB
- Volume
- 137
- Category
- Article
- ISSN
- 0009-2614
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β¦ Synopsis
Third-harmonic generation and multiphoton ionisation were simultaneously monitored at several pressures in Kr gas following excitation by a strongly focused dye laser, tunable over the range 338 to 350 nm. The results indicate that the multiphoton ionisation signals due to the nf [ l/2] autoionising series of Kr and the III* band of IQ1 are strongly enhanced by the third-harmonic radiation in the vacuum ultraviolet.
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