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Thermodynamic Enantioface-Binding Selectivities of Monosubstituted Alkenes to a Highly Discriminating Chiral Transition -Metal Lewis Acid; equilibration of diastereoisomeric (cyclopentadienyl)(alkene)(nitrosyl)(triphenylphosphine)rhenium complexes ([Re(η5–C5H5)(CH2 = CHR)(NO) (PPh3)]+BF)

✍ Scribed by Tang-Sheng Peng; Atta M. Arif; John A. Gladysz


Publisher
John Wiley and Sons
Year
1992
Tongue
German
Weight
1015 KB
Volume
75
Category
Article
ISSN
0018-019X

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✦ Synopsis


Reactions of monosubstituted alkenes RCH=CH, and [Re(q5-C,H5)(CH2CI,)(NO)(PPh3)]+BF; give complexes ([Re(q5-C5Hs)(CH2=CHR)(NO)(PPh,)l+BF; (la-g) in 63-99 %I yields as mixtures of (RS,SR)-and (RR,SS)-diastereoisomers ( l a (R