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Theoretical study of hydrogenated buckminsterfullerene derivatives with benzenoid rings, C60H60–66n (n= 1–8)

✍ Scribed by A. Rathna; Jayaraman Chandrasekhar


Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
730 KB
Volume
206
Category
Article
ISSN
0009-2614

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✦ Synopsis


The equilibrium geometries, heats of formation, and harmonic vibrational frequencies of hydrogenated buckminsterfullerene derivatives CsOH60_6n containing l-8 benzenaid units were computed using MNDO and AM1 methods. Although the Hessian indices indicate that all such structures are true minima, the T symmetry structure of C6&36 with four benzene rings is calculated to be the best prospect for experimental characterization. The relative stabilities of the various derivatives are principally controlled by angle strain at the sp* and sp" carbon atoms.