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Theoretical studies on the Mo-catalyzed asymmetric intramolecular Pauson-Khand-type [2 + 2 + 1] cycloadditions of 3-allyloxy-1-propynylphosphonates

✍ Scribed by Qingxi Meng, Ming Li


Book ID
118789941
Publisher
Springer-Verlag
Year
2012
Tongue
English
Weight
976 KB
Volume
18
Category
Article
ISSN
1610-2940

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The intramolecular 1,3-dipolar cycloaddition reactions of chiral morpholinone-derived azomethine ylides with tethered alkenes and alkynes have been investigated by semi-empirical methods and ab initio quantum mechanics. The observed ecient direction of the asymmetric induction in the 1,3-dipolar cyc