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Theoretical challenge to the X-ray structure determination of dichloronitronium ion (“inorganic phosgene”) Cl2NO+

✍ Scribed by Martin Brumm; Gernot Frenking; Wolfram Koch


Publisher
Elsevier Science
Year
1991
Tongue
English
Weight
381 KB
Volume
182
Category
Article
ISSN
0009-2614

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✦ Synopsis


Ab initio calculations predict that the N-O interatomic distance in &NO+, 1, is I, 16 t 0.03 A and suggest that the experimental value of I .30-l .32 A obtained by X-ray structure determination is probably erroneous. ' To whom correspondence should be addressed. *' The calculations have been performed using the Convex and IBM versions ofthe program packages GAUSSIAN 86 and 90